We propose encoding a qubit in a two-level subspace spanned by the lowest -orbital state in the excited valley of an anisotropic quantum dot and the excited -orbital in the ground valley, which we dub the qubit. There is an avoided crossing between these states due to valley-orbit coupling (VOC) induced by alloy disorder, enabling complete single-qubit control using baseband electrical control of the dot anisotropy. We find that `sweet spots’ exist at specific dot orientations where the instantaneous eigenstates are first-order insensitive to charge noise. Using a phenomenological two-level fluctuator (TLF) dipole noise model, we estimate an average dephasing time of and a quality factor of . Alternatively, encoding in the -orbital states in the ground valley near the isotropic dot point, we show that one can induce a similar sweet spot via an out-of-plane magnetic field. Finally, we find that two-qubit gates for the qubit are mediated by the quadrupole-quadrupole Coulomb interaction and can be electrically tuned from zero to by adjusting the relative orientation of the anisotropic dots, providing a novel pathway towards scalable quantum computation.

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