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Entangling gates of trapped ions are typically mediated by collective motional degrees of freedom. Weak coupling between qubit and motional degrees of freedom and the resulting harmonic dynamics give access to a broad range of gate schemes, but also impose strict limitations on achievable gate times. In this paper, we devise optimally designed driving schemes for the realization of fast, high-fidelity entangling gates mediated by anharmonic dynamics. The driving can also be optimized to achieve resilience to multiple system imperfections, and the anharmonicity in the motional dynamics can be used to enhance such resilience.

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