The production of two longitudinally polarized bosons is measured using proton-proton collision data recorded by the ATLAS experiment at a center-of-mass energy TeV and with an integrated luminosity of 164 fb. The candidate events are reconstructed using two same-flavor opposite-charge electron or muon pairs. The polarization fractions of the boson pair are measured inclusively in the fiducial phase space and also in two regions of the four-lepton invariant mass, and the results are consistent with the Standard Model predictions. After a statistical combination with a previous measurement at TeV, the first observation of the production of two simultaneously longitudinally polarized bosons is obtained, with observed and expected significances of 6.5 and 5.6 standard deviations, respectively.

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