All-optical magnetization control in CrI${}_3$ monolayers: a microscopic theory

Bright excitons in ferromagnetic monolayers CrI${}_3$ efficiently interact with lattice magnetization, which makes possible all-optical resonant magnetization control in this material. Using the combination of ab-initio simulations within Bethe-Salpeter approach, semiconductor Bloch equations and Landau-Lifshitz equations, we construct a microscopic theory of this effect. Solving numerically the resulting system of the coupled equations describing the dynamics of atomic spins and spins of the excitons, we demonstrate the possibility of a tunable control of macroscopic magnetization of a sample.