For any group , the Gorenstein homological dimension is defined to be the Gorenstein flat dimension of the coefficient ring , which is considered as an -module with trivial group action. We prove that if and only if the Gorenstein flat dimension of any -module is finite, if and only if there exists an -pure -monic with being -flat and , where is a commutative ring with finite Gorenstein weak global dimension. As applications, properties of on subgroup, quotient group, extension of groups as well as Weyl group are investigated. Moreover, we compare the relations between some invariants such as , , , , and Gorenstein projective, Gorenstein flat and PGF dimensions of -modules; a sufficient condition for Gorenstein projective-flat problem over group rings is given.

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