We prove the existence of nonconstant harmonic maps of optimal regularity from an arbitrary closed manifold of dimension to any closed, non-aspherical manifold containing no stable minimal two-spheres. In particular, this gives the first general existence result for harmonic maps from higher-dimensional manifolds to a large class of positively curved targets. In the special case of the round spheres , , we obtain a distinguished family of nonconstant harmonic maps of index at most , with singular set of codimension at least for sufficiently large. Furthermore, if , we show that these smooth harmonic maps stabilize as becomes large, and correspond to the solutions of an eigenvalue optimization problem on , generalizing the conformal maximization of the first Laplace eigenvalue on surfaces.

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