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The hexadecapole deformation () of the U nucleus has not been determined because its effect is overwhelmed by those from the nucleus’ large quadrupole deformation () in nuclear electric transition measurements. In this Letter, we identify the nonlinear response of the hexadecapole anisotropy to ellipticity in relativistic U+ U collisions that is solely sensitive to and insensitive to . We demonstrate this by state-of-the-art hydrodynamic calculations and discuss the prospects of discovering the of U in heavy-ion data at the Relativistic Heavy Ion Collider.

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