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In this paper, we mainly provide a new approache to construct Hom-Hopf algebras. For this, we introduce and study the notion of a left -Hom-crossed product structure as a generalization of -Hom-smash product structure. Then one combines this -Hom-crossed product structure and a left -Hom-smash coproduct structure to build Radford -biproduct theorem. Finally, we study Hom admissible mappping system to characterize this Radford -biproduct structure.

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