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All known examples of simply-connected gradient Kähler-Ricci soliton in real dimension four are toric, and the symmetry is intrinsically related to the potential function and the scalar curvature . In this article, we consider the case that and are functionally dependent and deduce a complete classification, while the independence case is addressed elsewhere. The main theorem recovers all known examples of cohomogeneity one symmetry. We also discover a connection to the theory of isoparametric functions and contact geometry. Indeed, a key ingredient is a new characterization for a deformed Sasakian structure generalizing a classical result.

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