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This paper combines explicit local calculations with covering arguments to prove the unboundedness above and below (in a logarithmic sense) of the Donaldson-Hitchin functionals on 4-forms, 3-forms and 4-forms, over compact manifolds (or, more generally, orbifolds) with boundary. In addition, the Donaldson-Hitchin functional on 3-forms over compact manifolds (or orbifolds) with boundary is shown to be unbounded below. As scholia, the critical points of the functionals on 4-forms, 3-forms and 4-forms are shown to be saddles, and initial conditions of the Laplacian coflow which do not lead to convergent solutions are shown to be dense.

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