We study the classical compilation of quantum circuits for the preparation of matrix product states (MPS), which are quantum states of low entanglement with an efficient classical description. Our algorithm represents a near-term alternative to previous sequential approaches by reverse application of a disentangler, which can be found by minimizing bipartite entanglement measures after the application of a layer of parameterized disentangling gates. Since a successful disentangler is expected to decrease the bond dimension on average, such a layer-by-layer optimization remains classically efficient even for deep circuits. Additionally, as the Schmidt coefficients of all bonds are locally accessible through the canonical - form of an MPS, the optimization algorithm can be heavily parallelized. We discuss guarantees and limitations to trainability and show numerical results for ground states of one-dimensional, local Hamiltonians as well as artificially spread out entanglement among multiple qubits using error correcting codes.

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