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Using collision data corresponding to an integrated luminosity of 10.6 fb collected at center-of-mass energies between 4.258 and 4.681 GeV with the BESIII detector at the BEPCII collider, we search for the charmonium-like hybrid via and decays for the first time. No significant signal is observed and the upper limits on the Born cross sections for both processes are set at the 90% confidence level.

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