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We investigate the boundedness of ``vertical’’ Littlewood–Paley–Stein square functions for the nonlocal fractional discrete Laplacian on the lattice , where the underlying graphs are not locally finite. When , we prove the boundedness of the square function by exploring the corresponding Markov jump process and applying the martingale inequality. When , we consider a modified version of the square function and prove its boundedness through a careful in on the generalized carré du champ operator. A counterexample is constructed to show that it is necessary to consider the modified version. Moreover, we extend the study to a class of nonlocal Schrödinger operators for .

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