Measurements of jet substructure in Pb+Pb collisions provide key insights into the mechanism of jet quenching in the hot and dense QCD medium created in these collisions. This Letter presents a measurement of the suppression of large-radius jets with a radius parameter of and its dependence on the jet substructure. The measurement uses 1.72 nb of Pb+Pb data and 255 pb of data, both at TeV, recorded with the ATLAS detector at the Large Hadron Collider. Large-radius jets are reconstructed by reclustering calorimetric jets and are measured for transverse momentum above GeV. Jet substructure is evaluated using charged-particle tracks, and the overall level of jet suppression is quantified using the jet nuclear modification factor (). The jet is measured as a function of jet , the charged splitting scale (), and the angular separation () of two leading sub-jets. The jet gradually decreases with increasing , implying significantly stronger suppression of large-radius jets with larger splitting scale. The jet gradually decreases for in the range and then remains consistent with a constant for . The observed significant dependence of jet suppression on the jet substructure will provide new insights into its role in the quenching process.

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