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High-resolution collinear laser spectroscopy of neutron-rich actinium has been performed at TRIUMF’s isotope separator and accelerator facility ISAC. By probing the ionic transition, the hyperfine structures and optical isotope shifts in Ac have been measured. This allows precise determinations of the changes in mean-square charge radii, magnetic dipole moments, and electric quadrupole moments of these actinium isotopes. The improved precision of charge radii and magnetic moments clears the ambiguity in the odd-even staggering from previous studies. The electric quadrupole moments of Ac are determined for the first time.

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