We present [NII] 205 m fine structure line observations of three submillimeter galaxies (SMGs) and three quasar host galaxies at 4z6 using the Institut de radioastronomie millimétrique (IRAM) interferometer. The [NII] emission is detected in three sources, and we report detections of the underlying dust continuum emission in all sources. The observed [NII]-to-infrared luminosity ratio spans at least 0.5 dex for our sources. Comparing our estimates with sources detected in the [NII] 205 m at similar redshifts shows that the overall [NII]-to-IR luminosity ratio spans over a dex in magnitude from L/L ~ 10 - 10 and follows the trend of the so-called [NII] fine structure line deficit observed in (ultra)-luminous infrared galaxies in the local Universe. The [CII]-to-[NII] luminosity ratio is >10 for most of our sources, indicating that the bulk of the [CII] 158 m line emission (f([CII])>75%) arises from the neutral medium. From our analysis, we do not find significant differences in the [NII] 205 m emission and the respective ratios between SMGs and QSOs, suggesting a negligible contribution to the boosting of [NII] 205 m emission due to the active galactic nucleus (AGN) photoionization. Future investigations involving other fine structure lines and optical diagnostics will provide further insight into a suite of ionized medium properties and reveal the diversity between AGN and non-AGN environments.

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