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Let be a sub-Laplacian on a two-step stratified Lie group of topological dimension . We prove new -spectral multiplier estimates under the sharp regularity condition in settings where the group structure of is degenerate, extending previously known results for the non-degenerate case. Our results include variants of the free two-step nilpotent group on three generators and Heisenberg-Reiter groups. The proof combines restriction type estimates with a detailed analysis of the sub-Riemannian geometry of . A key novelty of our approach is the use of a refined spectral decomposition into caps on the unit sphere in the center of the Lie group.

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