Plane-selective manipulations of nuclear spin qubits in a three-dimensional optical tweezer array

One of the central challenges for a practical fault-tolerant quantum computer is scalability. A three-dimensional structure of optical tweezer arrays offers the potential for scaling up neutral atom processors. However, coherent local operations, essential for quantum error correction, have yet to be explored for this platform. Here, we demonstrate plane-by-plane initialization of nuclear spin qubits of ${}^{171}\mathrm{Y}\mathrm{b}$ atoms in a three-dimensional atom array and plane-dependent coherent temporal evolution of qubits, as well as plane-selective qubit manipulation by exploiting the plane-selective excitation of the atoms from the ${}^1{S}_0$ to the ${}^3{P}_2$ state. This plane-selective manipulation technique paves the way for quantum computing and quantum simulation in three-dimensional multilayer architectures.