Neutron Scattering Studies on Magnetic Structure of the Double-Layered Manganite La_{2-2x}Sr_{1+2x}Mn_2O_7 ($0.30\le x\le 0.50$)

Systematic powder diffraction studies have been carried out to establish the magnetic phase diagram of La_{2-2x}Sr_{1+2x}Mn_2O_7 (LSMO327) in a wide hall concentration range ($0.30\le x\le 0.50$), using the HERMES diffractometer. LSMO327 exhibits a planar ferromagnetic structure for $0.32\le x\le 0.38$ at low temperatures. A finite canting angle between planar magnetic moments on neighboring planes starts appearing around $x\sim 0.40$ and reaches 180${}^{\circ }$ (A-type antiferromagnet) at x=0.48. At x=0.30, on the other hand, the magnetic moments are aligned parallel to the c-axis.