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Measurements on a multilayer two-dimensional electron system (2DES) near Landau level filling =1 reveal the disappearance of the nuclear spin contribution to the heat capacity as the ratio between the Zeeman and Coulomb energies exceeds a critical value 0.04. This disappearance suggests the vanishing of the Skyrmion-mediated coupling between the lattice and the nuclear spins as the spin excitations of the 2DES make a transition from Skyrmions to single spin-flips above . Our experimental is smaller than the calculated =0.054 for an ideal 2DES; we discuss possible origins of this discrepancy.

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