Quantitative Determination of the Adiabatic Condition Using Force-Detected Nuclear Magnetic Resonance

The adiabatic condition governing cyclic adiabatic inversion of proton spins in a micron-sized ammonium chloride crystal was studied using room temperature nuclear magnetic resonance force microscopy. A systematic degradation of signal-to-noise was observed as the adiabatic condition became violated. A theory of adiabatic following applicable to cyclic adiabatic inversion is reviewed and implemented to quantitatively determine an adiabaticity threshold $(\gamma H_1{)}^2\mathrm{/}({\omega }_{osc}\mathrm{\Omega })=6.0$ from our experimental results.