Giant perpendicular Edelstein polarization in 2D compensated magnets via bichromatic Floquet driving

While unconventional $p$-wave magnets can generate nonrelativistic Edelstein polarizations, spin-group symmetries strictly forbid these responses in unconventional magnets with higher-order harmonics, such as $d$-wave altermagnets. Here, we demonstrate that combining Rashba spin-orbit coupling with bichromatic Floquet driving activates giant perpendicular Edelstein polarizations (PEPs) across 2D altermagnets and broader classes of unconventional spin-polarized magnets – a feat monochromatic driving cannot achieve. By dynamically breaking two-fold rotational symmetry, the two-frequency drive (including bilinear, bicircular, and circular-linear configurations) induces a stray-field-free in-plane Zeeman-like field that generates orbitally dominated PEPs (0.5–1.5 ${\mu }_{\mathrm{B}}$). This massive response is governed by universal selection rules tied to the system’s magnetic parity and the second beam’s harmonics. These emergent PEPs provide a powerful mechanism for perpendicular memory writing.