In this paper, we first study infinitesimal deformations of a Lie conformal algebra and a Lie conformal algebra with a module (called an pair), which lead to the notions of Nijenhuis operator on the Lie conformal algebra and Nijenhuis structure on the pair, respectively. Then by adding compatibility conditions between Nijenhuis structures and -operators, we introduce the notion of an $ N N$-operators on a Lie conformal algebra can be characterized by Nijenhuis operators on Lie conformal algebras. Finally, we introduce the notions of conformal -matrix-Nijenhuis structure and symplectic-Nijenhuis structure on the Lie conformal algebra and study their relations.

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