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We calculate the Picard group of generic (very general) spectral varieties living in the total space of a very ample line bundle over an algebraically closed field of odd characteristics or characteristic 0. We follow the strategy of Ravindra and Srinivas [RS06,RS09] via formal Picard groups. As an application, we calculate the generic fibers of Hitchin systems over a smooth quintic surface of Picard number 1.

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