Two-dimensional (2D) magnetic materials with strong magnetostriction are interesting systems for strain-tuning the magnetization, enabling potential for realizing spintronic and nanomagnetic devices. Realizing this potential requires understanding of the magneto-mechanical coupling in the 2D limit. In this work, we suspend thin CrGeTe layers, creating nanomechanical membrane resonators. We probe its mechanical and magnetic properties as a function of temperature and strain. Pronounced signatures of magneto-elastic coupling are observed in the temperature-dependent resonance frequency of these membranes near . We further utilize CrGeTe in heterostructures with thin layers of WSe and FePS, which have positive thermal expansion coefficients, to compensate the negative thermal expansion coefficient of CrGeTe and quantitatively probe the corresponding . Finally, we induce a strain of in a suspended heterostructure via electrostatic force and demonstrate a resulting enhancement of by K in the absence of an external magnetic field.

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