This paper presents measurements of top-antitop quark pair () production in association with additional -jets. The analysis utilises 140 fb of proton-proton collision data collected with the ATLAS detector at the Large Hadron Collider at a centre-of-mass energy of 13 TeV. Fiducial cross-sections are extracted in a final state featuring one electron and one muon, with at least three or four -jets. Results are presented at the particle level for both integrated cross-sections and normalised differential cross-sections, as functions of global event properties, jet kinematics, and -jet pair properties. Observable quantities characterising -jets originating from the top quark decay and additional -jets are also measured at the particle level, after correcting for detector effects. The measured integrated fiducial cross-sections are consistent with predictions from various next-to-leading-order matrix element calculations matched to a parton shower within the uncertainties of the predictions. State-of-the-art theoretical predictions are compared with the differential measurements; none of them simultaneously describes all observables. Differences between any two predictions are smaller than the measurement uncertainties for most observables.

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