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We use the technique of invariant frames to study a left invariant spray structure on a Lie group, and calculate its S-curvature and Riemann curvature, which generalizes the corresponding formulae in homogeneous Finsler geometry. Using the canonical bi-invariant Berwald spray structure as the reference, any left invariant spray structure can be associated with a spray vector field on the Lie algebra. We find the correspondence between geodesics for a left invariant spray structure and the inverse integral curves of its spray vector field. As an application for this correspondence, we provide an alternative proof for Landsberg Conjecture in the case of homogeneous Finsler surfaces.

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