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We report on the observation of the spin-exchange dynamics of atoms in the ground state and in the metastable state . We implement the mixed-dimensional two-orbital system using a near-resonant and magic-wavelength optical lattices, where the and atoms are itinerant in a one-dimensional tube and localized in three dimensions, respectively. By exploiting an optical Stern-Gerlach method, we observe the spin depolarization of the atoms induced by the spin-exchange interaction with the atom. Our work could open the way to the quantum simulation of the Kondo effect.

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