We present measurements of bulk radiocontaminants in the high-resistivity silicon CCDs from the DAMIC at SNOLAB experiment. We utilize the exquisite spatial resolution of CCDs to discriminate between and decays, and to search with high efficiency for the spatially-correlated decays of various radioisotope sequences. Using spatially-correlated decays, we measure a bulk radioactive contamination of Si in the CCDs of $140 \pm 30$ Bq/kg, and place an upper limit on bulk Pb of $< 160~\mu\alpha< 11$ Bq/kg (0.9 ppt) on U and of $< 7.3$ Bq/kg (1.8 ppt) on Th. The ability of DAMIC CCDs to identify and reject spatially-coincident backgrounds, particularly from Si, has significant implications for the next generation of silicon-based dark matter experiments, where ’s from Si decay will likely be a dominant background. This capability demonstrates the readiness of the CCD technology to achieve kg-scale dark matter sensitivity.

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