We report the first electron neutrino cross section measurements on argon, based on data collected by the ArgoNeuT experiment running in the GeV-scale NuMI beamline at Fermilab. A flux-averaged total and a lepton angle differential cross section are extracted using 13 and events identified with fully-automated selection and reconstruction. We employ electromagnetic-induced shower characterization and analysis tools developed to identify -like events among complex interaction topologies present in ArgoNeuT data ($\langle E_{\bar{\nu}e} \rangle = 4.3\langle E{\nu_e} \rangle = 10.5$ GeV). The techniques are widely applicable to searches for electron-flavor appearance at short- and long-baseline using liquid argon time projection chamber technology. Notably, the data-driven studies of GeV-scale interactions presented in this Letter probe an energy regime relevant for future DUNE oscillation physics.

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