Through 2.6 GeV U irradiations, we have induced bimodal splayed columnar defects in BaKFeAs single crystals with splay angles, $\pm 5 ^\circ\pm 10 ^\circ\pm 15 ^\circ\pm 20 ^\circ$. Critical current densities through magnetization measurements were carefully evaluated, where a splay angle of brought about the highest . Mageto-optical images close to indicates highly anisotropic discontinuity lines in the remnant state, and with anisotropy increasing with greater splay angles. Moreover, amongst those with splayed columnar defects, anomalous non-monotonic field dependences of and with an extrema at some fraction of the matching field are observed. We discuss that such enhancement arises from a field-driven coupling transition in which intervortex interactions reorganize the vortex structure to be accommodated into columnar defects, thereby increasing pinning at higher fields.

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