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We report on the demonstration of Doppler-free spectroscopy of metastable Sr atoms using a hollow cathode lamp (HCL). We employed a custom Sr HCL which is filled with a mixture of 0.5-Torr Ne and 0.5-Torr Xe as a buffer gas to suppress velocity changing collisions and increase the populations in all the metastable states. We performed frequency-modulation spectroscopy for the , , , and transitions with sufficient signal to noise ratios for laser frequency stabilization. We also observed the hyperfine transitions of of . This method would greatly facilitate laser cooling of Sr.

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