Let be the single-electron fiber Hamiltonians of the massless Nelson model at total momentum and infrared cut-off . We establish detailed regularity properties of the corresponding -particle ground state wave functions as functions of and . In particular, we show that where is a numerical constant, is a positive function of the maximal admissible coupling constant which satisfies and is the (approximate) characteristic function of the energy region between the infrared cut-off and the ultraviolet cut-off . While the analysis of the first derivative is relatively straightforward, the second derivative requires a new strategy. By solving a non-commutative recurrence relation we derive a novel formula for with improved infrared properties. In this representation is amenable to sharp estimates obtained by iterative analytic perturbation theory in part II of this series of papers. The bounds stated above are instrumental for scattering theory of two electrons in the Nelson model, as explained in part I of this series.

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