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This paper deals with characterizing the freeness and asymptotic freeness of free multiple integrals with respect to a free Brownian motion or a free Poisson process. We obtain three characterizations of freeness, in terms of contraction operators, covariance conditions, and free Malliavin gradients. We show how these characterizations can be used in order to obtain limit theorems, transfer principles, and asymptotic properties of converging sequences.

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