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In the present paper, we study Neumaier Cayley graphs. First, we give a criterion for a Cayley graph to be a Neumaier graph with a spread given by the cosets of a subgroup. Further, we construct a new infinite family of Neumaier Cayley graphs of unbounded nexus. Finally, we provide an algorithm for enumerating Neumaier Cayley graphs and computational results obtained by this algorithm.

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