The dense Galactic Center environment is expected to host compact binary inspirals detectable by future space-borne gravitational wave (GW) observatories (e.g., LISA, TianQin, Taiji) in the millihertz band. Aided by information from these facilities, next-generation ground-based GW detectors (e.g., Cosmic Explorer, Einstein Telescope) can potentially capture gravitational radiation in the hectohertz band from rapidly spinning neutron star (NS) components in such binaries. These Galactic Center systems are thus anticipated to act as dual-line (i.e., low-frequency inspiral and high-frequency spin) GW sources. However, the formation channels of these systems remain largely unexplored. In this , we propose that the von Zeipel-Lidov-Kozai (ZLK) effect can enhance the formation of dual-line GW sources in hierarchical triples involving the Galactic supermassive black hole, Sgr A*. We show that ZLK-driven oscillations in the eccentricity and inclination of the inner binary can modulate the GW emission from both the binary inspiral and the individual NS spins. This effect boosts the expected dual-line source count by a factor of , from rare to in 4 years, making dual-line observations substantially more probable. Our results demonstrate that the ZLK effect may provide an important formation channel for Galactic dual-line GW sources.

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