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Using general-relativistic hydrodynamical simulations, we show that merging binary neutron stars can form hypermassive neutrons stars that undergo the one-arm spiral instability. We study the particular case of a dynamical capture merger where the stars have a small spin, as may arise in globular clusters, and focus on an equal-mass scenario where the spins are aligned with the orbital angular momentum. We find that this instability develops when post-merger fluid vortices lead to the generation of a toroidal remnant - a configuration whose maximum density occurs in a ring around the center-of-mass

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