In this Letter, we propose a strategy to extract information on the hierarchical amplitude pair in singly Cabibbo-suppressed (SCS) charmed baryon two-body decays, with a dominant amplitude proportional to from tree operators and sub-leading one proportional to from both penguin and tree contributions. The coexistence of these two amplitudes is essential for generating nonzero CP violation (CPV) effects. Since the amplitude is strongly suppressed, its experimental determination is highly challenging. However, by exploiting SU(3) flavor symmetry, which relates the well-measured Cabibbo-favored (CF) amplitudes to the SCS tree amplitudes, information on the amplitude can be extracted. Using current experimental data, a conservative analysis yields amplitudes can be as large as about of the corresponding tree amplitudes with a significance of . In addition, the Lee-Yang parameters of these decays provide an independent probe of this elusive term. We further identify two golden decay channels, and , which are particularly well suited for experimental studies of CPV.

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