We investigate unnatural-parity high-spin states in neutron-rich Cr and Fe
isotopes using large-scale shell-model calculations. These shell-model
calculations are carried out within the model space of fp-shell + 0g9/2
- 1d5/2 orbits with the truncation allowing 1ℏω excitation of a
neutron. The effective Hamiltonian consists of GXPF1Br for fp-shell orbits
and VMU with a modification for the other parts. The present
shell-model calculations can describe and predict the energy levels of both
natural- and unnatural-parity states up to the high-spin states in Cr and Fe
isotopes with N≤35. The total energy surfaces present the prolate
deformations on the whole and indicate that the excitation of one neutron into
the 0g9/2 orbit plays the role of enhancing the prolate deformation. For
the positive(unnatural)-parity states in odd-mass Cr and Fe isotopes, their
energy levels and prolate deformations indicate the decoupling limit of the
particle-plus-rotor model. The sharp drop of the 9/21+ levels in going
from N=29 to N=35 in odd-mass Cr and Fe isotopes is explained by the Fermi
surface approaching the ν0g9/2 orbit.