We investigate the imprint of clustering on initial spin fluctuations in relativistic and collisions at ~TeV. Utilizing configurations from Nuclear Lattice Effective Field Theory (NLEFT) and phenomenological -cluster models within a Monte-Carlo Glauber framework, we compute the event-by-event variance of the initial net spin polarization. We find that the strong short-range spin–isospin correlations characteristic of clusters lead to a significant suppression of spin fluctuations compared to a spherical Woods–Saxon baseline with uncorrelated spins. By constructing a scaled fluctuation observable that accounts for trivial finite-size effects, we demonstrate that this suppression exhibits a non-monotonic centrality dependence sensitive to the detailed cluster geometry. Furthermore, we propose the ratio of scaled spin fluctuations between and systems as a robust probe. Our results predict distinct percent-level deviations from the baseline for clustered nuclei, suggesting that measurements of final-state -hyperon spin correlations can provide novel constraints on the ground-state spin structure of light nuclei.

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