We evaluate pairwise correlations using ground state wave functions for He and He obtained by no-core shell model (NCSM) calculations with the Daejeon16 nucleon-nucleon interaction plus Coulomb interaction, to characterize the structures of these two systems. We demonstrate that two-nucleon spatial correlations, specifically the pair-number operator and the square-separation operator projected on two-body spin and isospin -components encode important details of the halo structure of He. We also analyze the single-particle state occupancies and the two-body state occupancies for the ground state of He and He. Our results indicate that the two valence neutrons in the ground state of He dominantly form a spin-singlet configuration. The rms pair separations between core nucleons and halo neutrons of He is about 80% larger than pair separations within the swollen and off-centered “ core”. We show that this off-centering effect is primarily responsible for the observed increase in point-proton radius in He relative to He.

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