Polycrystalline samples of the isostructural alloys UNi1-xCoxSi2 (0 <= x <=
- were studied by means of x-ray powder diffraction, magnetization, electrical
resistivity and specific heat measurements, at temperatures down to 2 K and in
magnetic fields up to 5 T. The experimental data revealed an evolution from
strongly anisotropic ferromagnetism with pronounced Kondo effect, observed for
the alloys with x < 0.98 and being gradually suppressed with rising Co-content,
to spin-glass-like states with dominant spin fluctuations, seen for the sample
with x = 0.98. Extrapolation of the value of TC(x) yields a critical
concentration xc = 1, at which the magnetic ordering entirely disappears. This
finding is in line with preliminary data collected for stoichiometric UCoSi2.