A generalized perturbative approach for the computation of nonlinear scattering problems

We present a perturbative technique for modeling the scattering of light by a nonlinear material. This approach eliminates the need for an iterative algorithm to solve the fully coupled nonlinear problem. We demonstrate its effectiveness in the cases of a nonlinear anisotropic slab and a nonlinear periodic crystal, both illuminated by a plane wave under conical incidence and arbitrary polarization. Quantitative comparisons of the accuracy and computational time with our previously published rigorous model are provided.