Interactions derived from effective field theories of quantum chromodynamics have thus far failed to bind calcium nuclei beyond neutron number , while nuclear density functionals typically place the neutron dripline near Ca, at . We present the chiral interaction NLO, a combination of two- and three-nucleon potentials at fourth and third chiral order, respectively, with low-energy constants optimized using emulator-accelerated fits to few- and many-body data. This interaction accurately reproduces binding energies and charge radii of key nuclei with mass number to , important excited states, and nuclear matter near saturation. Using ab-initio methods, we find that the calcium two-neutron dripline extends to Ca.

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