Understanding the astrophysical origins of binary black holes requires accurate and flexible modeling of multi-dimensional population properties. In this paper, using a data-driven framework based on binned Gaussian processes, we characterize the joint distribution of BBH primary masses, mass ratios, and effective inspiral spins. We identify three distinct subpopulations in the GWTC-4 sample of observations and investigate their astrophysical origins. We find that only one of the three subpopulations exhibits the peak, which is characterized by a strong preference for equal mass systems and isotropic spin orientations. Our inferred distributions are consistent with a predominantly dynamical origin of this feature. By comparing with theoretical simulations, we further show that the subpopulation that exhibits the peak can exclusively comprise dynamically assembled systems in globular clusters, specifically if black hole birth spins are in the range~, whereas the other two subpopulations require substantial contributions from alternative formation channels. We constrain the on the merger rate of BBHs in globular clusters to be , which is consistent with theoretical predictions. We conclude that dynamical formation in globular clusters remains a strong candidate for the origin of this excess near and that more data and targeted parametric models are necessary to rigorously establish this interpretation.

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