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Often considered in numerical simulations related to the control of quantum systems, the so-called monotonic schemes have not been so far much studied from the functional analysis point of view. Yet, these procedures provide an efficient constructive method for solving a certain class of optimal control problems. This paper aims both at extending the results already available about these algorithms in the finite dimensional case (i.e., the time-discretized case) and at completing those of the continuous case. This paper starts with some results about the regularity of a functional related to a wide class of model in quantum chemistry. Those enable us to extend an inequality due to

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