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This article aims to raise awareness within the ESO astronomical community of the scientific opportunities offered by the upcoming Cherenkov Telescope Array, CTAO, highlighting cases where combining millimetre/submillimetre capabilities of the Atacama Large Millimeter / submillimeter Array, ALMA with the CTAO’s very high energy, TeV, observations enables new avenues for discovery. Many astrophysical sources and environments exhibit emission processes detectable in both regimes; however, the synergies extend beyond shared emission mechanisms and include broader physical processes and observational connections linking millimetre, submillimetre and TeV energies.

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